Controlling multidimensional off-resonant-Raman and infrared vibrational spectroscopy by finite pulse band shapes.
نویسنده
چکیده
Closed expressions are derived which incorporate pulse shaping effects in femtosecond nonlinear optical signals involving various combinations of temporally well-separated vibrationally resonant infrared and electronically off-resonant Raman pulses. Combinations of broadband and narrow band pulses that yield multidimensional extensions of coherent anti-Stokes Raman and sum frequency generation spectroscopy are presented.
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ورودعنوان ژورنال:
- The Journal of chemical physics
دوره 130 5 شماره
صفحات -
تاریخ انتشار 2009